57Fe NMR and Mössbauer study of peculiarities of long-range magnetic ordering in Fe3C cementite
- 作者: Mikhalev K.N.1, Suvorkova Y.V.1, Germov A.Y.1, Prokopyev D.A.1, Goloborodsky B.Y.1, Novikov S.I.1, Uimin M.A.1, Yermakov A.E.1,2, Gaviko V.S.1
-
隶属关系:
- M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
- Ural Federal University, Ekaterinburg, 620002 Russia
- 期: 卷 126, 编号 6 (2025)
- 页面: 643-650
- 栏目: ЭЛЕКТРИЧЕСКИЕ И МАГНИТНЫЕ СВОЙСТВА
- URL: https://bakhtiniada.ru/0015-3230/article/view/322659
- DOI: https://doi.org/10.31857/S0015323025060016
- ID: 322659
如何引用文章
详细
The 57Fe NMR spectra and relaxation times in θ-Fe3C cementite in the region of long-range magnetic order were obtained and analyzed. The values of hyperfine magnetic fields for two nonequivalent positions of iron atoms in the structure (Pnma) of this compound and their evolution in the temperature range from 4.2 to 350 K were determined. From the analysis of the 57Fe Mossbauer spectra obtained at T = 295 K, the components of the electric field gradient tensor and the values of hyperfine fields were determined.
作者简介
K. Mikhalev
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
Ye. Suvorkova
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
A. Germov
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
D. Prokopyev
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
B. Goloborodsky
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
S. Novikov
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
M. Uimin
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
A. Yermakov
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia; Ural Federal University, Ekaterinburg, 620002 Russia
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia; Ekaterinburg, 620002 Russia
V. Gaviko
M.N. Mikheev Institute of Metal Physics of Ural Branch of Russian Academy of Sciences, Ekaterinburg, 620108 Russia
编辑信件的主要联系方式.
Email: e.v.suvorkova@mail.ru
Ekaterinburg, 620108 Russia
参考
- Цементит в углеродистых сталях: коллектив. монография / Под ред. В.М. Счастливцева. Екатеринбург: УМЦ УПИ, 2017. 380 с.
- Yelsukov E.P., Barinov V.A., Ovetchkin L.V. Synthesis of disordered Fe3C alloy by mechanical alloying of iron powder with liquid hydrocarbon (toluene) // J. Mater. Sci. Lett. 1992. V. 11. No. 10. P. 662–663.
- Ekstrom H.C., Adcock W.A. A new iron carbide in hydrocarbon synthesis catalys // J. Amer. Chem. Soc. 1950. V. 72. P. 1042–1051.
- Fasiska E.J., Jeffrey G.A. On the cementite structure // Acta Crystal. 1965. V. 19. No. 3. P. 463–471.
- Razumovskiy V.I., Ghosh G. A first-principles study of cementite (Fe3C) and its alloyed counterparts: Structural properties, stability, and electronic structure // Comput. Mater. Sci. 2015. V. 110. P. 169–181.
- Germov A.Y., Prokopyev D.A., Mikhalev K.N., Goloborodskiy B.Y., Uimin M.A., Yermakov A.E., Konev A.S., Minin A.S., Novikov S.I., Gaviko V.S., Murzakaev A.M. Quantitative phase analysis of magnetic Fe@C nanoparticles // Mater. Today Commun. 2021. V. 27. P. 102382.
- Баринов В.А., Цурин В.А., Казанцев В.А., Суриков В.Т. Карбонизация α-Fe при механосинтезе // ФММ. 2014. Т. 115. С. 57.
- Le Caer G., Dubois J.M., Senateur J.P. Etude par spectrométrie Mössbauer des carbures de Fer Fe3C et Fe5C2 // J. Solid State Chem. 1976. V. 19. No. 1. P. 19–28.
- David B., Schneeweiss O., Dumitrache F., Fleaca C., Alexandresc, R., Morjan I. Powders with superparamagnetic Fe3C particles studied with Mössbauer spectrometry // J. Phys. Conf. Ser. 2010. V. 217. No. 1. P. 012097.
- Медведева Н.И., Карькина Л.Е., Ивановский А.Л. Влияние примеси хрома на электронную структуру цементита Fe3C // ФТТ. 2006. Т. 48. С. 17.
- Hirano S., Tajima S. Synthesis and Magnetic Properties of Iron Carbide (Fe3C) // J. Jpn. Soc. Powder Powder Metall. 1990. V. 37. No. 3. P. 421–425.
- Choe H., Terai T., Fukuda T., Kakeshita T., Yamamoto S., Yonemura M. Easy axis of magnetization of Fe3C prepared by an electrolytic extraction method // J. Magn. Magn. Mater. 2016. V. 417. P. 1–5.
- Ron M., Mathalone Z. Hyperfine Interactions of Fe57 in Fe3C // Phys. Rev. B. 1971. V. 4. No. 3. P. 774–777.
- Bernas H., Campbell I.A., Fruchart R. Electronic exchange and the Mössbauer effect in iron-based interstitial compounds // J. Phys. Chem. Solids. 1967. V. 28. P. 17–24.
- Liu X.W., Zhao S., Meng Y., Peng Q., Dearden A.K., Huo C.F., Yang Y., Li Y.W., Wen X.D. Mössbauer spectroscopy of iron carbides: From prediction to experimental confirmation // Sci. Rep. 2016. V. 6. No. 1. P. 26184.
- Туров Е.А., Петров М.П. Ядерный магнитный резонанс в ферро- и антиферромагнетиках. М.: Наука, 1969. 260 с.
- Shaham M., Barak J., El-Hanany U., Warren W.W. NMR study of the 3d ferromagnetic metals: Critical region and paramagnetic phase // Phys. Rev. B. 1980. V. 22. No. 11. P. 5400–5419.
- Mikhalev K., Verkhovskii S., Gerashenko A., Mirmelstein A., Bobrovskii V., Kumagai K., Furukawa Y., D’yachkowa T., Zainulin Yu. Temperature dependence of sublattice magnetization of the infinite-layer antiferromagnet SrCuO2 // Phys. Rev. B. 2004. V. 69. P. 132415–132418.
- Arzhnikov A.K., Dobysheva L.V. Structural peculiarities of plastically-deformed cementite and their influence on magnetic characteristics and Mossbauer parameters // Solid State Commun. 2008. V. 146. No. 1–2. P. 102–104.
- Kuz’min M.D., Richter M., Yaresko A.N. Factors determining the shape of the temperature dependence of the spontaneous magnetization of a ferromagnet // Phys. Rev. B. Condens. Matter Mater. Phys. 2006. V. 73. No. 10. P. 100401.
- Kuz’min M.D. Skokov K.P., Diop L.V.B., Radulov I.A., Gutfleisch O. Exchange stiffness of ferromagnets // Eur. Phys. J. Plus. 2020. V. 135. No. 3. P. 1–8.
- Абрагам А. Ядерный магнетизм. Москва: ИИЛ, 1963. 551 с.
- Лапина О.Б., Хабибулин Д.Ф., Шубин А.А. Современные возможности ЯМР-спектроскопии твердого тела квадрупольных ядер. Журнал структурной химии // Журнал структурной химии. 2010. Т. 51. С. 33.
- Germov A.Y., Prokopyev D.A., Konev A.S., Uimin M.A., Minin A.S., Yermakov A.E., Goloborodsky B.Yu., Kurmachev I.A., Suvorkova Ye.V. NMR and Mossbauer studies of core–shell FeCo@ C ferromagnetic nanoparticles near the superparamagnetic transition // J. Magn. Magn. Mater. 2023. V. 588. P. 171391.
- Hah H.Y. Mössbauer Spectroscopy of Iron Oxide Nanoparticles: Materials for Biomedical Applications, PhD diss. University of Tennessee, 2018. 65 p.
- Вонсовский С.В., Туров Е.А. Динамические и кинетические свойства магнетиков. М.: Наука, 1986. 248 с.
补充文件
